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Anand, Naween; Barry, Kevin; Neu, Jennifer N.; Graf, David E.; Huang, Qing; Zhou, Haidong; Siegrist, Theo; Changlani, Hitesh J.; Beekman, Christianne (, Nature Communications)Abstract The single-ion anisotropy and magnetic interactions in spin-ice systems give rise to unusual non-collinear spin textures, such as Pauling states and magnetic monopoles. The effective spin correlation strength (Jeff) determines the relative energies of the different spin-ice states. With this work, we display the capability of capacitive torque magnetometry in characterizing the magneto-chemical potential associated with monopole formation. We build a magnetic phase diagram of Ho2Ti2O7, and show that the magneto-chemical potential depends on the spin sublattice (αorβ), i.e., the Pauling state, involved in the transition. Monte Carlo simulations using the dipolar-spin-ice Hamiltonian support our findings of a sublattice-dependent magneto-chemical potential, but the model underestimates theJefffor theβ-sublattice. Additional simulations, including next-nearest neighbor interactions (J2), show that long-range exchange terms in the Hamiltonian are needed to describe the measurements. This demonstrates that torque magnetometry provides a sensitive test forJeffand the spin-spin interactions that contribute to it.more » « less
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Barry, Kevin; Zhang, Biwen; Anand, Naween; Xin, Yan; Vailionis, Arturas; Neu, Jennifer; Heikes, Colin; Cochran, Charis; Zhou, Haidong; Qiu, Y.; et al (, Physical Review Materials)
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